References
Lakowicz, J. R. Principles of Fluorescence Spectroscopy 3rd edn (Springer US, New York, 2007).
Moerner, W. & Orrit, M. Illuminating single molecules in condensed matter. Science 283, 1670–1676 (1999).
Schatz, G. C. & Ratner, M. A. Quantum Mechanics in Chemistry (Courier Corp., New York, 1993).
Herzberg, G. Infrared and Raman Spectra of Polyatomic Molecules Vol. 2 (D. Van Nostrand, New York, 1945).
Nie, S. & Emory, S. R. Probing single molecules and single nanoparticles by surface-enhanced Raman scattering. Science 275, 1102–1106 (1997).
Seilmeier, A., Kaiser, W., Laubereau, A. & Fischer, S. A novel spectroscopy using ultrafast two-pulse excitation of large polyatomic molecules. Chem. Phys. Lett. 58, 225–229 (1978).
Hübner, H.-J., Wörner, M., Kaiser, W. & Seilmeier, A. Subpicosecond vibrational relaxation of skeletal modes in polyatomic molecules. Chem. Phys. Lett. 182, 315–320 (1991).
Mastron, J. N. & Tokmakoff, A. Two-photon-excited fluorescence-encoded infrared spectroscopy. J. Phys. Chem. A 120, 9178–9187 (2016).
Cheng, J. & Xie, X. Coherent anti-Stokes Raman scattering microscopy: instrumentation, theory, and applications. J. Phys. Chem. B 108, 827–840 (2004).
See AlsoSemrock Optical FiltersMin, W., Freudiger, C. W., Lu, S. & Xie, X. S. Coherent nonlinear optical imaging: beyond fluorescence microscopy. Annu. Rev. Phys. Chem. 62, 507–530 (2011).
Lee, S., Nguyen, D. & Wright, J. Double resonance excitation of fluorescence by stimulated Raman scattering. Appl. Spectrosc. 37, 472–474 (1983).
Shim, S., Stuart, C. M. & Mathies, R. A. Resonance Raman cross‐sections and vibronic analysis of Rhodamine 6G from broadband stimulated Raman spectroscopy. ChemPhysChem 9, 697–699 (2008).
Wei, L. & Min, W. Electronic preresonance stimulated Raman scattering microscopy. J. Phys. Chem. Lett. 9, 4294–4301 (2018).
Etchegoin, P. G., Le, Ru,E. C. & Meyer, M. Evidence of natural isotopic distribution from single-molecule SERS. J. Am. Chem. Soc. 131, 2713–2716 (2009).
Min, W. et al. Imaging chromophores with undetectable fluorescence by stimulated emission microscopy. Nature 461, 1105–1109 (2009).
Sperber, P., Spangler, W., Meier, B. & Penzkofer, A. Experimental and theoretical investigation of tunable picosecond pulse generation in longitudinally pumped dye laser generators and amplifiers. Opt. Quant. Electron. 20, 395–431 (1988).
Wei, L. et al. Super-multiplex vibrational imaging. Nature 544, 465–470 (2017).
Dean, K. M. & Palmer, A. E. Advances in fluorescence labeling strategies for dynamic cellular imaging. Nat. Chem. Biol. 10, 512–523 (2014).
Kneipp, K. et al. Single molecule detection using surface-enhanced Raman scattering (SERS). Phys. Rev. Lett. 78, 1667–1670 (1997).
Sonntag, M. D. et al. Single-molecule tip-enhanced Raman spectroscopy. J. Phys. Chem. C 116, 478–483 (2011).
Yampolsky, S. et al. Seeing a single molecule vibrate through time-resolved coherent anti-Stokes Raman scattering. Nat. Photon. 8, 650–656 (2014).
Zhang, Y. et al. Coherent anti-Stokes Raman scattering with single-molecule sensitivity using a plasmonic Fano resonance. Nat. Commun. 5, 4424 (2014).
Mahmoudi, M. et al. Protein–nanoparticle interactions: opportunities and challenges. Chem. Rev. 111, 5610–5637 (2011).
Macklin, J., Trautman, J., Harris, T. & Brus, L. Imaging and time-resolved spectroscopy of single molecules at an interface. Science 272, 255–258 (1996).
Nie, S., Chiu, D. T. & Zare, R. N. Probing individual molecules with confocal fluorescence microscopy. Science 266, 1018–1021 (1994).
Kukura, P., Celebrano, M., Renn, A. & Sandoghdar, V. Single-molecule sensitivity in optical absorption at room temperature. J. Phys. Chem. Lett. 1, 3323–3327 (2010).
Chong, S., Min, W. & Xie, X. S. Ground-state depletion microscopy: detection sensitivity of single-molecule optical absorption at room temperature. J. Phys. Chem. Lett. 1, 3316–3322 (2010).
Gaiduk, A., Yorulmaz, M., Ruijgrok, P. & Orrit, M. Room-temperature detection of a single molecule’s absorption by photothermal contrast. Science 330, 353–356 (2010).
Zrimsek, A. et al. Single-molecule chemistry with surface- and tip-enhanced Raman spectroscopy. Chem. Rev. 117, 7583–7613 (2017).
Winterhalder, M., Zumbusch, A., Lippitz, M. & Orrit, M. Toward far-field vibrational spectroscopy of single molecules at room temperature. J. Phys. Chem. B 115, 5425–5430 (2011).
Brinks, D. et al. Ultrafast dynamics of single molecules. Chem. Soc. Rev. 43, 2476–2491 (2014).
Kukura, P., McCamant, D. W. & Mathies, R. A. Femtosecond stimulated Raman spectroscopy. Annu. Rev. Phys. Chem. 58, 461–488 (2007).
Siegman, A. E. Lasers. (University Science Books, Mill Valley, CA, 1986).
Wright, J. C. Double resonance excitation of fluorescence in the condensed phase—an alternative to Infrared, Raman, and fluorescence spectroscopy. Appl. Spectrosc. 34, 151–157 (1980).
Zipfel, W. R., Williams, R. M. & Webb, W. W. Nonlinear magic: multiphoton microscopy in the biosciences. Nat. Biotechnol. 21, 1369–1377 (2003).